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Inicio  /  Coatings  /  Vol: 13 Par: 6 (2023)  /  Artículo
ARTÍCULO
TITULO

Orthorhombic YBa2Cu3O7-d Superconductor with TiO2 Nanoparticle Addition: Crystal Structure, Electric Resistivity, and AC Susceptibility

Fatma Barood    
Mohd Mustafa Awang Kechik    
Tan Sin Tee    
Chen Soo Kien    
Lim Kean Pah    
Kai Jeat Hong    
Abdul Halim Shaari    
Hussein Baqiah    
Muhammad Khalis Abdul Karim    
Muhammad Kashfi Shabdin    
Khairul Khaizi Mohd Shariff    
Azhan Hashim    
Nurbaisyatul Ermiza Suhaimi and Muralidhar Miryala    

Resumen

This article reports the effect of a nanoscale addition of TiO2 on the structure and superconducting parameters of the high-temperature superconductor YBa2Cu3O7-d (Y123). Polycrystalline compounds of Y123 with different percentages of TiO2, x = 0.0, 0.2, 0.4, 0.6, 0.8, and 1.0, were fabricated using the thermal treatment method. An analysis using X-ray diffraction confirmed the formation of Y123 phases for all composite samples. Field-emission scanning electron microscopy (FESEM) analysis revealed the growth of grain size and decrease in porosity, with a sign of partial melting of grains for the samples with TiO2 addition. The magnetic and electric transport properties were investigated using AC susceptibility measurement and the four-probe method, respectively. It was observed that the superconducting transition temperature, Tc-onset, for a pure sample determined by ACS and 4PP was 95.6 K and 95.4 K, respectively. These values were found to decrease with the addition of TiO2, while the superconducting transition (?Tc) improved with TiO2 addition except for the sample at x = 0.2 wt.%, which showed the broadest transition width. The sharpest superconducting transition (?Tc) was observed for the sample at x = 1.0 wt.%, indicating that the addition of TiO2 nanoparticles is expected to serve as artificial pinning centres and strengthen the connection among the grains in the Y123 ceramic.

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