3.1. Computational Analysis
A shock wave itself exerts limited influence on the breakup of sub-millimeter liquid droplets. Instead, the primary factor is the significant relative velocity generated in the flow field surrounding a droplet after a shock wave’s passage, initiating a sequence of deformations and fragmentations [
33]. In practice, a droplet experiences acceleration under the influence of air that is thousands of times greater than gravitational acceleration. Consequently, gravity’s effect is usually neglected in the description of droplet evolution and quantitative parameter analysis [
34]. When dimensionally analyzing droplet evolution, we can assess interactions between various parameters. The dimensionless windward displacement, denoted by
, is defined as the ratio of the distance moved along the airflow from the beginning of the windward to the initial droplet diameter (
). The dimensionless transverse deformation width, denoted as
, signifies the ratio of the width of the transverse deformation along the vertical airflow direction during the droplet’s evolution to the initial diameter (
). Furthermore, the dimensionless axial deformation width, denoted as
, is defined as the ratio of the axial deformation width in the direction of the airflow propagation to the initial diameter (
), as illustrated in
Figure 8. To eliminate the influence of airflow-related parameters, the following formulas were used to nondimensionalize the fragmentation time:
where
t is the dimensional time,
is the initial diameter of the droplet, and
and
represent the densities of the liquid phase and the gas phase, respectively. The moment when the shock wave contacts the droplet is defined as time zero.
In the simplified representation shown in
Figure 9, the computational domain model depicts a left-to-right propagating shock wave. A sub-millimeter liquid droplet is symmetrically positioned on the central axis. The shock tube’s cross-sectional area is 60 mm × 60 mm, and the experimental section has a length of 500 mm. This study exclusively examined the physical attributes of the flow field around sub-millimeter liquid droplets, eliminating the need for a numerical simulation of the entire shock tube structure. The simplified calculation spatial domain size was chosen such that
,
, and
. This approach not only mitigated the influence of reflected waves but also conserved computational resources, to some extent. Given the high flow field symmetry, a one-quarter model was selected for the numerical simulation. “Symmetry” boundary conditions were imposed on the two central planes containing sub-millimeter liquid droplets. At the left boundary of the computational domain, pressure inlet boundary condition was applied and at the right boundary, a pressure outlet was assigned. Other boundary conditions, which included the top and back boundaries of the computational domain, were set to symmetry. The flow field used structured grids, and the sub-millimeter liquid droplet section employed a grid gradient adaptation to improve the computational efficiency. Dynamic grid adaptation based on phase fraction gradient was implemented inANSYS Fluent V20.2. This involved adjusting the mesh dynamically by refining regions with high gradient values and coarsening regions with low gradient values. To achieve this, the refinement thresholds were set to refine the grids in areas with large gradients, while coarsening thresholds were set to revert the mesh in areas with small gradients. For unsteady flow environments, it was essential to control the entire computational time by standardizing the gradient values. In the scaling method, the “Scale by Global Maximum” option was applied. Finally, for the phase fraction gradient adaptation, specific refinement and coarsening values were provided, with a refinement value of 0.06, a coarsening value of 0.05, and a maximum refinement level that was set to 4. Grid refinement was automatically conducted during the calculations based on the liquid volume fraction gradient to achieve an accurate solution domain. Furthermore, under these thermodynamic conditions, the environmental pressure in the flow field exceeded the saturated vapor pressure of the water. Consequently, during the sub-millimeter liquid droplet deformation and breakup, no phase change occurred, and it could be assumed that the gas–liquid two-phase was immiscible.
In this research, the multiphase flow model selected was the VOF (volume-of-fluid) model due to its excellent mass conservation properties and effective interface capturing capabilities. It can accurately describe mass transfer in the fluid and interface diffusion [
14,
32,
35]. This method is based on the idea of treating liquid and gas as a single two-component medium. Within the computational domain, the spatial distribution of the liquid phase was characterized by a step function, denoted as F (x, y, z, t), with values that ranged between 0 and 1. If the entire computational grid was occupied by the liquid phase, F (x, y, z, t) was equal to one, if it was entirely occupied by the gas phase, F (x, y, z, t) was equal to zero. In cases where both the liquid and gas phases coexisted within the computational grid, 0 < F (x, y, z, t) < 1. As the value of F (x, y, z, t) changed over time, solving the transport equation for the volume fraction of the liquid phase within the grid allowed for the determination of the distribution of the two-phase system. This, in turn, enabled the tracking of the evolution of the liquid phase interface.
Our simulation calculations assumed that the liquid phase was incompressible and treated the gas phase as an ideal gas governed by the gas state equation. Gravity effects were not taken into consideration. The governing equations included the continuity equation, momentum equation, and energy equation, as follows:
In the above continuity equation, the subscripts
and
correspond to the gas phase and liquid phase, respectively, and
represents velocity,
is a Cartesian coordinate component, and
and
denote the volume fractions of the liquid phase and gas phase, respectively, which were needed to satisfy Equation (8).
In the momentum equation,
is the molecular stress tensor and
is the Reynolds stress tensor whose components have the following form:
where
is the velocity relaxation time,
is the surface tension,
is the molecular dynamic viscosity,
is the turbulent viscosity coefficient,
denotes the gas phase, and
denotes the liquid phase.
In the above energy equation,
E is the total energy,
keff is the effective thermal transmittance, and the effective viscous stress tensor,
τeff,ij, is given as follows:
In numerical simulations, where the gas phase is considered an ideal gas, it is imperative to augment the ideal gas state equation to complete the control equations mentioned above as follows:
where
p represents the gas pressure, R is the gas constant, and
T stands for the temperature.
3.2. Computational Model Establishment and Verification
The numerical calculations were conducted using the industrial simulation software ANSYS Fluent V20.2. It has been successfully applied to past aerodynamic fragmentation studies on liquid droplets under shock wave impacts [2726,3234]. Turbulent flow simulations were conducted by applying the k-w SST model in the context of unsteady Reynolds-averaged Navier–Stokes (RANS) equations. The solution method involved the use of a pressure-based coupled solver with the pressure–velocity coupling resolved through the PISO algorithm, which has been recognized for its efficiency in achieving convergence with fewer iterations. Spatial discretization of the pressure field was performed using the robust PRESTO! scheme, which is well suited for multiphase flow problems. The density, momentum, and turbulent kinetic energy were discretized with the third-order MUSCL scheme. The initial configuration of the sub-millimeter liquid droplets and the flow field was established with the Patch function. This function partitioned the computational domain into regions with uniform high- and low-pressure parameters to set the initial conditions for the propagating shock waves. The initial parameters on both sides of the shock waves were determined following the shock tube principles. Based on the flow conditions, a constant time step size of s was defined for the explicit transient simulations.
Various grid densities were utilized to evaluate the grid independence in constructing the fluid domain, ensuring that the density had no impact on the computational outcomes. The non-dimensional displacement of the sub-millimeter droplets on the windward side was compared at a Mach number of 2.12 using various grid densities. CFD I utilized 1,686,528 cells, CFD II employed 2,502,892 cells, and CFD III featured 3,015,726 cells.
Figure 10 demonstrates that there were no significant differences in the non-dimensional displacements of the sub-millimeter droplets over time for the three grid densities. To ensure both manageable computational demands and the complete capturing of the gas–liquid interface evolution, this study chose the grid density of CFD II for the subsequent three-dimensional numerical simulations of the sub-millimeter droplet aerodynamic breakup.
In order to validate our numerical simulation method and ensure the accuracy of the subsequent computational results, we applied this method to calculate the dimensionless transverse deformation widths for two specific parameter conditions, C2 (Ma = 1.17 and
= 0.9) and D1 (Ma = 1.36 and
= 0.84), as defined by Shi [
26] for vertical airflow. The results are depicted in
Figure 11. A comparison between these numerical simulation results and the experimental data highlighted the improved consistency when employing the numerical simulation method introduced in this paper. Nevertheless, due to the inherent uncertainties in the experimental measurements, there was no definitive value for the liquid phase volume fraction,
, that best fit the data. This variability contributed, to some extent, to the disparity between the numerical simulation results and the experimental outcomes.
3.3. Results and Discussion
Figure 12 presents the morphological evolution of the windward and leeward surfaces at eight discrete time instances from the dimensionless times 0 to 1.497. The shapes corresponded to liquid phase isosurfaces with volume fractions of
= 0.99, 0.50, and 0.01 at
Ma = 2.12 operating conditions. Under these operating conditions, the airflow attained a supersonic state with the post-shock Mach number
. This supersonic environment amplified the instant deformation and aerodynamic breakup of the sub-millimeter liquid droplets. During the initial stage (
), the sub-millimeter liquid droplets remained largely undeformed. Surface disturbances arising from the instability began to develop gradually. At this point, the droplets could be approximated as rigid bodies with no significant axial displacements along the airflow direction. When
, sub-millimeter liquid droplets experienced initial distortion and deformation. The windward side retained a relatively spherical shape, while the leeward side was rapidly compressed into a flat shape. Subsequently, when
, vortical structures continuously developed and expanded on the leeward sides of the sub-millimeter liquid droplets due to the airflow, resulting in the formation of noticeable cavities in the leeward regions. Concurrently, the sub-millimeter liquid droplets underwent the strong shearing effect of the K–H instability. Small-scale liquid sheets and sub-droplets continually detached from the equatorial regions and downstream of the leeward sides of the droplets. High-speed airflow accelerated and stretched them away from the parent droplets. This process, influenced by flow instability, resulted in the thinning and gradual development of ligaments from the thinner parts of the liquid sheets. Over time, these ligaments became finer, and their collisions further contributed to the droplets’ fragmentation into smaller liquid droplets. Consequently, in the later stages of fragmentation (
), a widespread distribution of sub-droplets became apparent in the downstream regions. Through a comprehensive examination of the sub-millimeter liquid droplet characteristics, it became evident that the deformation and breakup of the sub-millimeter liquid droplets in a supersonic airflow environment aligned with the SIE breakup mechanism as proposed by Theofanous [
11].
The comparison between the numerical simulation results and the experimental visualizations at corresponding time points is presented in
Figure 13. The figure illustrates a close correspondence between the deformation and breakup morphologies of the sub-millimeter liquid droplets obtained through the numerical simulations and the experimental photographs. Additionally,
Figure 14 provides a parameter comparison, depicting the dimensionless transverse deformation widths of the sub-millimeter liquid droplets in the vertical airflow direction over time. The results revealed good qualitative agreement between the numerical simulations and the experimental measurements, underscoring the effectiveness of our numerical simulation method in capturing the interface evolution during the sub-millimeter liquid droplet breakup process.
Figure 15 displays the streamline, velocity contours, and pressure contours illustrating the deformation and fragmentation processes of the sub-millimeter liquid droplets subjected to shock wave conditions with an
Ma value of 2.12. Small surface waves formed on the windward surfaces and propagated toward the equators from the initial moment. On the leeward surfaces of the sub-millimeter liquid droplets, airflow separation occurred, resulting in the formation of small vortexes. At this point, the airflow near the windward surfaces demonstrated high pressures and low velocities. The pressures on the windward surfaces were not uniform, and the surface waves created high-pressure stagnation points on the windward sides by impeding the airflow behind the waves. In the equatorial regions of the sub-millimeter liquid droplets, low pressures and high velocities prevailed, with the highest airflow speed observed at this position. When considering the droplets’ stagnation states, it became evident that the maximum tangential velocity differences between the gas and liquid phases occurred on the equatorial planes, resulting in the onset of Kelvin–Helmholtz instability. Subsequently, due to the significantly lower pressures in the equatorial regions compared to the pressures at the front and rear stagnation points, the sub-millimeter liquid droplets underwent flattening. This flattening reduced the curvatures on the windward sides of the droplets, leading to increased variations in the airflow velocities as they traversed the droplets. This, in turn, promoted the continuous growth of vortices on the leeward sides and propelled the propagation of the surface waves towards the equatorial planes. When examining
Figure 12, it is evident that the sub-millimeter liquid droplets expanded laterally in the vertical airflow direction, while the leeward regions adopted concave shapes, causing sub-droplets to continually detach from the vicinity of the equatorial planes.
The velocity contours revealed flame-like tails extending in the airflow direction on the leeward sides of the sub-millimeter liquid droplets. In the influence of the vortices, there were observable annular low-speed regions in the middles of the velocity distributions on the leeward sides, corresponding to the outer vortex regions. Finally, the flow fields and vortex structures on the leeward sides continue to develop and became more complex. The main sizes and masses of the droplets decreased continuously due to the detachment of small droplets, while the annular low-speed regions at the tails enlarged continuously due to the expansion of the vortexes.
A quantitative investigation into the deformation process of the sub-millimeter liquid droplets was subsequently carried out.
Figure 16 illustrates the dimensionless axial deformation widths aligned with the flow direction and the dimensionless transverse deformation widths aligned with vertical airflow over time. The results are presented for volume fractions of 0.01, 0.5, and 0.99. The axial widths of the sub-millimeter liquid droplets decreased approximately linearly with time in the airflow direction, while the evolution of the transverse widths in the vertical airflow direction underwent the following two stages: a slow flattening deformation stage and a strong shear stretching deformation stage, which aligned with the characteristics observed in the numerical simulations for the sub-millimeter liquid droplets’ deformation and fragmentation, as shown in
Figure 12.